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The study suggests a simple approach to improve phase transition properties and ferroelectricity of a typical ferroelectric metal-organic framework of [NH 4 ][Zn(HCOO) 3 ] (AmZn) using silicon dioxides nanoparticles (nSiO 2 ). It is shown that the first-order transition type of AmZn is not changed under the influence of nSiO 2 . Moreover, the phase transition temperature of AmZn significantly increased with increasing the nSiO 2  content from 0 to 40 wt%. Besides, the addition of small nSiO 2  content (&lt; 11%) led to rising spontaneous saturation and remnant polarizations. The study also indicated difficulties in obtaining the saturation P-E loops at high nSiO 2  content.

Phase transition and ferroelectricity of composites based on ferroelectric metal-organic framework of [NH 4 ][Zn(HCOO) 3 ]