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An efficient and facile synthesis for 2-aminobenzimidazoles and 2-aminobenzoxazoles has been reported. Thioureas prepared from the reaction of  o -phenylenediamines or 2-aminophenols and isothiocyanate derivatives, underwent desulfurization reaction smoothly under mild conditions in the presence of Cu(OAc) 2 , and afforded a variety of  N -heterocyclic compounds in moderate to good yields.

Cu(OAc) 2 mediated mild synthesis of 2-aminobenzimidazoles and 2-aminobenzoxazoles