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The chiral 2-amino-4 H -chromene derivatives were obtained from 2-alkyl-substituted phenol derivatives in moderate to high yields with excellent enantioselectivities through one-pot cascade via C–H oxidation/Michael addition/ring closure sequences using a binaphthyl-modified organocatalyst with low catalyst loading (1.25 mol%).

Enantioselective one-pot synthesis of 2-amino-4 H -chromenes via C−H oxidation and Michael addition/ring closure sequences