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Laser induced fluorescence and dispersed fluorescence spectroscopy was used to investigate the  B5 Π -1  –  X5 Π -1  system of the chromium monosulfide molecule. The rotational constant and Λ-doubling parameter of  B5 Π -1  (v′ = 7), as a newly observed upper vibrational level, were obtained from the rotationally resolved laser excitation spectrum. For the ground  X5 Π -1  state, the vibrational frequency and vibrational anharmonicity constant were experimentally determined for the first time from the dispersed fluorescence spectrum. In addition, the lifetimes of the upper  B5 Π -1  (v′ = 0 − 7) levels were measured by fitting the time-dependent fluorescence decay.

Laser-induced fluorescence spectroscopy of the B 5 Π -1 – X 5 Π -1 system of the chromium monosulfide molecule