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The dynamic effect concerning small mixing of first-excited state to ground state due to the ligand vibration (which can bring about a twinkling tetrahedral change from compression to elongation) is introduced to calculate the gyromagnetic (g) factors of the second compressed tetragonal molybdenum (V) tetrahedral center in the light-irradiated lead molybdate crystal. The computed results agree well with the observed values, and the large deviation of the observed  g//  from  g e(≈2.0023, the free electron  g  factor) is therefore interpreted. The outcomes (particularly, the percentage in time for the twinkling tetrahedral change from compression to elongation) are discussed.

Dynamic effect to gyromagnetic factors of the compressed tetragonal molybdenum (V) tetrahedral center in the light-irradiated lead molybdate crystal