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Theband has been identified and measured in the laboratory spectrum of the CD molecule for the first time. The emission from the discharge was observed with a high accuracy dispersive optical spectroscopy technique using a plane-grating spectrograph and recorded by a photomultiplier tube. In total, 99 ro-vibronic frequencies were measured with an absolute accuracy of about cm. In the following work, we present the results of the combined analysis of the current experimental data and the(0−0) [Szajna et al., J. Mol. Spectrosc.  324 , 48–52 (2016)] and(0−0) [Herzberg and Johns, Astrophys. J.  158 , 399–417 (1969)] bands of CD. The resulting data, compared to those from the earlier measurements, present more accurate molecular constants for the  v  = 0 vibrational level of the and states. The parameters of the Λ-doubling ( p ,  q ) of the( v  = 0) level were obtained for the first time. The current observations and analysis have become a basis to discuss the possible detection of the CD radical in the interstellar medium by the,+andspectral lines of theband in the 3880 Å region.

The emission spectroscopy of the astrophysically significant B 2 Σ − –X 2 Π system of CD: further investigation