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We describe methods for the production of spin-polarised H and D atoms from the IR-excitation and photodissociation of molecular beams of HBr, HI, and NH 3  isotopes, including optical excitation schemes with partial hyperfine resolution. We discuss the extent to which the production rates may approach the IR-laser production rates of, and how the production rates of conventional methods ofmay be surpassed significantly.

Macroscopic production of spin-polarised hydrogen atoms from the IR-excitation and photodissociation of molecular beams