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Significance Carbon dioxide electroreduction may constitute a key technology in coming years to valorize CO2 as high value-added chemicals such as hydrocarbons and a way to store intermittent solar energy durably. Based on readily available technologies, systems combining a photovoltaic (PV) cell with an electrolyzer cell (EC) for CO2 reduction to hydrocarbons are likely to constitute a key strategy for tackling this challenge. However, a low-cost, sustainable, and highly efficient PV–EC system has yet to be developed. In this article, we show that this goal can be reached using a low-cost and easily processable perovskite photovoltaic minimodule combined to an electrolyzer device using the same Cu-based catalysts at both electrodes and in which all energy losses have been minimized.

Low-cost high-efficiency system for solar-driven conversion of CO 2 to hydrocarbons

Low-cost high-efficiency system for solar-driven conversion of CO ₂ to hydrocarbons