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We review the results from two experiments that used resonant four-wave mixing (RFWM) techniques to investigate double-resonance transitions in NO. In the first experiment, laserinduced grating decay curves that reveal quantum beats due to the hyperfine structure of the A 2Σ, υ' = 0 state were observed and interpreted. In the second, multistate interactions between the L 2II1/ 2,3/2, υ = 8 and Q 2II1/ 2,3/2, υ = 0 states were investigated, and new assignments were made. The results highlight the potential of RFWM techniques for probing excited-state physics.

Excited-state Structure and Dynamics of Nitric Oxide probed by Resonant Four-wave Mixing Techniques