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Niisanen et al.1 have reported equilibrium data for nickel@)-pn$ complexes in aqueous NaC104 media, I =.O.05-2.0~, and Carlson et a1.2 and Edwards3 have reported data for 0 . 5 ~ 1 KC1 (30") and 1~ KC1 (25") respectively. Basolo et al.4 have reported data for the nickel@)-pn and nickel@)-ibn complexes in aqueous KN03-Ba(N03)2, I = 0 . 6 5 ~ . There appear to be no other reported equilibrium data for nickel(n) complexes with C-alkylethylenediamines.3 This paper presents further data for the complexes with pn and ibn and the first data for complexes with eten; data are given for NaC104-Ba(C104)2 media in the ionic strength range 0 a04-0 3 5 ~ . The data reported are concentration quotients, K, = [NiL,]/[L][NiL,-11, and the thermodynamic formation constants KO, obtained by extrapolation of K, data to zero ionic strength.

Stabilities of nickel(II) complexes with some C-alkylethylenediamines