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has a significantly higher absolute magnitudes than that in methane (12.4*OS6 c/s)ls2 in agreement with the prediction made by Pople and Bothner-By.l Geminal coupling in 2,2,3,3-tetramethylbutane (Table 1) also appears to be higher than that in methane, but the difference is within the uncertainty of the measurements. In view of the high value of Jgem in tetramethylsilane, it may be possible that the magnitudes of Jgem in compounds of structure (CH,),X, where X = C, Ge, Sn, and H,D Isotope Effects from Differences between

Geminal interproton coupling constants in 2,2,3,3-tetramethylbutane and tetramethylsilane