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We determine the nucleation rates of hard spheres using brute-force moleculardynamics simulations. We overcome nucleation barriers of up to $28 k_B T$,leading to a rigorous test of nucleation rates obtained from rare-event methodsand classical nucleation theory. Our brute-force nucleation rates showexcellent agreement with umbrella sampling simulations by Filion et al. [J.Chem. Phys. 133, 244115 (2010)] and seeding simulations by Espinosa et al. [J.Chem. Phys. 144, 034501 (2016)].

Brute-force nucleation rates of hard spheres compared with rare-event methods and classical nucleation theory