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We introduce a minimal model of solid-forming anisotropic molecules thatdisplays, in thermal equilibrium, surface orientational order without bulkorientational order. The model reproduces the nonequilibrium behavior of recentexperiments in that a bulk nonequilibrium structure grown by depositioncontains regions of orientational order characteristic of the surfaceequilibrium. This order is deposited in general in a nonuniform way, because ofthe emergence of a growth-poisoning mechanism that causes equilibrated surfacesto grow slower than non-equilibrated surfaces. We use evolutionary methods todesign oscillatory protocols able to grow nonequilibrium structures withuniform order, demonstrating the potential of protocol design for thefabrication of this class of materials.

Deposition control of model glasses with surface-mediated orientational order