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The recent demonstration of MoSi2N4 and its exceptional stability to air,water, acid, and heat has generated intense interest in this family oftwo-dimensional (2D) materials. Among these materials, NbSi2N4, VSi2N4, andVSi2P4 are semiconducting, easy-plane ferromagnets with negligible in-planemagnetic anisotropy. They thus satisfy a necessary condition for exhibiting adissipationless spin superfluid mode. The Curie temperatures of monolayerVSi2P4 and VSi2N4 are determined to be above room temperature based on MonteCarlo and density functional theory calculations. The magnetic moments ofVSi2N4 can be switched from in-plane to out-of-plane by applying tensilebiaxial strain or electron doping.

Magnetic Properties of NbSi2N4, VSi2N4, and VSi2P4 Monolayers