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Large unsaturated magnetoresistance (XMR) with magnitude about 1000% isobserved in topological insulator candidate TaSe3 from our high field (up to 38T) measurements. Two oscillation modes, associated with one hole pocket and twoelectron pockets in the bulk, respectively, are detected from our Shubnikov-deHass (SdH) measurements, consistent with our first-principles calculations.With the detailed Hall measurements performed, our two-band model analysisexhibits an imperfect density ratio n_h/n_e closing 0.9 at T< 20 K , whichsuggests that the carrier compensations account for the XMR in TaSe3.

Large Magnetoresistance in Topological Insulator Candidate TaSe3