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Photoelectron circular dichroism (PECD) in different regimes of multiphotonionization of fenchone is studied theoretically using the time-dependent singlecenter method. In particular, we investigate the chiral response to theone-color multiphoton or strong-field ionization by circularly polarized 400and 814 nm optical laser pulses or 1850 nm infrared pulse. In addition, thebroadband ionization by short coherent circularly polarized 413-1240 nmspanning pulse is considered. Finally, the two-color ionization by thephase-locked 400 and 800 nm pulses, which are linearly polarized inmutually-orthogonal directions, is investigated. The present computationalresults on the one-color multiphoton ionization of fenchone are in agreementwith the available experimental data. For the ionization of fenchone bybroadband and bichromatic pulses, the present theoretical study predictssubstantial multiphoton PECDs.

Photoelectron circular dichroism in the multiphoton ionization by short laser pulses: III. Photoionization of fenchone in different regimes