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We have studied the structural stability of Sc-substituted rare earth (R)ferrites R1-xScxFeO3, and constructed a structural phase diagram for differentR and x. While RFeO3 and ScFeO3 adopt the orthorhombic and the bixbyitestructure respectively, the substituted compound R1-xScxFeO3 may be stable in adifferent structure. Specifically, for R0.5Sc0.5FeO3, the hexagonal structurecan be stable for small R, such as Lu and Yb, while the garnet structure isstable for larger R, such as Er and Ho. The formation of garnet structure ofthe R0.5Sc0.5FeO3 compounds which requires that Sc occupies both the rare earthand the Fe sites, is corroborated by their magnetic properties.

Structural phase diagram and magnetic properties of Sc-substituted rare earth ferrites R1-xScxFeO3 (R=Lu, Yb, Er, and Ho)