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The interface between organic semiconductor [OSC]/ferromagnetic [FM] materialcan exhibit ferromagnetism due to their orbital hybridization. Charge/spintransfer may occur from FM to OSC layer leading to the formation of`spinterface' i.e. the interface exhibiting a finite magnetic moment. In thiswork, the magnetic properties of Co/C$_{60}$ bilayer thin film have beenstudied to probe the interface between Co and C$_{60}$ layer. Polarized neutronreflectivity [PNR] measurement indicates that the thickness and moment of thespinterface are $\sim$ 2 $\pm$ 0.18 nm and 0.8 $\pm$ 0.2 $\mu_B$/cage,respectively. The comparison of the magnetization reversal between theCo/C$_{60}$ bilayer and the parent single layer Co thin film reveals thatspinterface modifies the domain microstructure. Further, the anisotropy of thebilayer system shows a significant enhancement ($\sim$ two times) in comparisonto its single layer counterpart which is probably due to an additionalinterfacial anisotropy arising from the orbital hybridization at theCo/C$_{60}$ interface.

Enhanced anisotropy and study of magnetization reversal in Co/C60 bilayer thin film