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Assembly of spherical colloidal particles into extended structures, includinglinear strings, in the absence of directional interparticle bondinginteractions or external perturbation could facilitate the design of newfunctional materials. Here, we use methods of inverse design to discoverisotropic pair potentials that promote the formation of single-stranded,polydisperse strings of colloids "colloidomers" as well as size-specific,compact colloidal clusters. Based on the designed potentials, a simple modelpair interaction with a short-range attraction and a longer-range repulsion isproposed which stabilizes a variety of different particle morphologiesincluding (i) dispersed fluid of monomers, (ii) ergodic short particle chainsas well as porous networks of percolated strings, (iii) compact clusters, and(iv) thick cylindrical structures including trihelical Bernal spirals.

Assembly of particle strings via isotropic potentials