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All TbNi2, TbMn2, and TbNi2Mn compounds exhibit the cubic Laves phase with AB2-typestructure in spite of the fact that the ratio of the Tb to transition-metal components in TbNi2Mn is1:3. Rietveld refinement indicates that in TbNi2Mn the Mn atoms are distributed on both the A (8a)and B (16d) sites. The values of the lattice constants were measured to be a¼14.348A ° (spacegroup F-43 m), 7.618A ° , and 7.158A ° (space group Fd-3 m) for TbNi2, TbMn2, and TbNi2Mn,respectively. The magnetic transition temperatures TC were found to be TC¼38K and TC¼148Kfor TbNi2 and TbNi2Mn, respectively, while two magnetic phase transitions are detected forTbMn2 at T1¼20K and T2¼49 K. Clear magnetic history effects in a low magnetic field areobserved in TbMn2 and TbNi2Mn. The magnetic entropy changes have been obtained. © 2014 AIP Publishing LLC

A comparative study of magnetic behaviors in TbNi2, TbMn2 and TbNi2Mn