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Time-resolved X-ray solution scattering is sensitive to global molecular structure andcan track the dynamics of chemical reactions. In this article, we review our recentstudies on triiodide ion (I3–) and molecular iodine (I2)in solution. For I3–, we elucidated the excitationwavelength-dependent photochemistry and the solvent-dependent ground-state structure. ForI2, by combining time-slicing scheme and deconvolution data analysis, wemapped out the progression of geminate recombination and the associated structural changein the solvent cage. With the aid of X-ray free electron lasers, even clearer observationof ultrafast chemical events will be made possible in the near future

structural dynamics

Topical Review: Molecular reaction and solvation visualized by time-resolved X-ray solution scattering: Structure, dynamics, and their solvent dependence