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We report a giant zero field cooled exchange bias (ZEB) effect (~0.65 T) inLa1.5Sr0.5CoMnO6 sample. Magnetic study has revealed a reentrant spin glass ~90K, phase separation to spin glass and ferromagnetic phases below 50 K andcanted antiferromagnetic transition ~10 K. A small conventional exchange bias(CEB) is established with the advent of spontaneous phase separation down to 10K. Giant ZEB and enhanced CEB effects are found only below 10 K and areattributed to the large unidirectional anisotropy at the interface ofisothermally field induced ferromagnetic phase and canted antiferromagneticbackground.

Giant zero field cooled spontaneous exchange bias effect in phase separated La1.5Sr0.5CoMnO6