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Bi2ZnOB2O6 nonlinear optical single crystals were grown by means of the Kyropoulos method from stoichiometric melt. The second and third harmonic generation (SHG/THG) of Bi2ZnOB2O6 crystals were investigated by the SHG/THG Maker fringes technique. Moreover, SHG microscopy studies were carried out providing two-dimensional SHG images as a function of the incident laser polarization. The high nonlinear optical efficiency combined with the possibility to grow high quality crystals make Bi2ZnOB2O6 an excellent candidate for photonic applications

Multifunctional Bi2ZnOB2O6 single crystals for second and third order nonlinear optical applications