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envelopes gave values of the ionic state bond lengths of (1.63560.005) and (1.64160.005) Å for the X 3S 2 and a 1D states of BrO1, respectively. The O1Br2 reaction was found to give a band at (10.2660.02) eV associated with a reaction product. Comparison of the results obtained for the Br1O3 reaction showed that it could not be assigned to ionization of BrO. Calculations of the first adiabatic ionization energies and Franck-Condon simulations of the vibrational envelopes of the first photoelectron bands of BrO 2 and Br2O and their isomers demonstrated that this band corresponds to the first ionization of OBrO, the BrO 2 1 (X 1A1)ˆBrO2(X 2 B1) ionization. Franck- Condon simulations were performed with the experimental geometry of BrO2(X ˜ 2 B1) but with different cationic state geometries. The simulated envelope which most closely matched the experimental envelope gave geometrical parameters of r e51.6135 Å and/OBrO5117.5° for the ionic state. © 2000 American Institute of Physics.@S0021-9606~00!00214-2#

A study of the BrO and BrO2 radicals with vacuum ultraviolet photoelectron spectroscopy