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A new disordered atom configuration in Fe2CrGa alloy has been created byball-milling method. This leads to a significant enhancement of the magneticmoment up to 3.2~3.9 {\mu}B and an increase of Curie temperature by about 200K, compared with the arc-melt samples. Combination of first-principlescalculations and experimental results reveals that Fe2CrGa alloy shouldcrystallize in Hg2CuTi based structure with different atomic disorders for thesamples prepared by different methods. It is addressed that magneticinteractions play a crucial role for the system to adopt such an atomicconfiguration which disobeys the empirical rule.

Disorder-induced significant enhancement in magnetization of ball-milled Fe2CrGa alloy