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By using laboratory x-ray photoemission spectroscopy (XPS) and hard x-rayphotoemission spectroscopy (HX-PES) at a synchrotron facility, we report anempirical semi-quantitative relationship between the valence/core-level x-rayphotoemission spectral weight and electrical conductivity inLa_{1-x}Sr_{x}MnO_{3} as a function of x. In the Mn 2p_{3/2} HX-PES spectra, weobserved the shoulder structure due to the Mn^{3+} well-screened state.However, the intensity at x=0.8 was too small to explain its higher electricalconductivity than x=0.0, which confirms our recent analysis on the Mn 2p_{3/2}XPS spectra. The near-Fermi level XPS spectral weight was found to be a measureof the variation of electrical conductivity with x in spite of a far lowerenergy resolution compared with the energy scale of the quasiparticle(coherent) peak because of the concurrent change of the coherent and incoherentspectral weight.

journal of applied physics

Empirical relationship between x-ray photoemission spectra and  electrical conductivity in a colossal magnetoresistive manganite  La_{1-x}Sr_{x}MnO_{3}