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Our lack of understanding of the factors that compensate energy defects in near resonant V-V energy transfer constrains our ability to accurately predict resonance widths and, thus, the overall importance of such processes. We have carried out one of the first truly state-to-state measurements of near resonant V-V energy transfer under single collision conditions, employing the crossed molecular beams, stimulated emission pumping technique. We have varied the energy defect ΔE for the process: NO

Rotational motion compensates the energy defect in near-resonant vibration–vibration energy transfer: A state-to-state study of NO(v)+N2O