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The temperature dependence of elastic, dielectric, and piezoelectricproperties of (65-x)Pb(Mg1/3Nb2/3)O3-xBaTiO335-PbTiO3 ceramics with x=0, 1, 2,3, and 4 was investigated. Compound with x=2 was found to exhibit a largepiezoelectric response (d31=-170 pC/N, d33=530 pC/N at 300 K). Particularly,its d31 value was nearly a constant over a temperature range from 185 to 360 K.A broad ferroelectric phase transition tuned by BaTiO3 doping was deduced fromthe dielectric constant, elastic compliance constant and Raman spectra. Thetemperature-stable piezoelectric response was attributed to the counter-balanceof contributions from the dielectric and elastic responses.

Large and temperature-independent piezoelectric response in Pb(Mg1/3Nb2/3)O3-BaTiO3-PbTiO3