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A detailed comparison of quasiclassical trajectory (QCT) and quantum mechanical (QM) reaction probabilities and differential cross sections for the H+D2→HD+D reaction at the collision energies of 0.54 and 1.29 eV has been carried out using the same potential energy surface. The theoretical simulation of the recently published experimental results is also reported. The comparisons made here demonstrate the level of agreement between QCT and QM approaches, as well as between theory and experiment for this reaction. © 1994 American Institute of Physics.Financed by the DGICYT of Spain under Grant No. PB92-0219-C03. GermanSpanish Scientific Exchange Program >Acciones Integradas>HA-074. At the University of Texas, this research was supported by the Robert Welch Foundation and the National Science Foundation. The German part was financed by the German Science Foundation under Grants No. WE 386/19 and SCHN 435/3 and by the Deutscher Akademischer Austauschdienst (Acciones Integradas) 322-AI-e-dr.Peer Reviewe

Quantum mechanical and quasiclassical calculations for the H+D2→HD+D reaction: Reaction probabilities and differential cross sections