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bending hot bands associated with the v4 fundamental. This constitutes the first characterization of the bending potential of C, . Excitation to u = 1’ of the Y, I (IT,, ) bending fundamental is accompanied by a huge increase (9.3%) in the rotational constant. Excitation from v = 1’ to v = 2’ of Y,~ results in an even larger increase ( 10.4%) in the rotational constant. The magnitude of these changes indicates extremely large amplitude bending motion about the central carbon atom, evidencing the predicted nonrigidity of C, . In addition, the v4 rotational transitions have been measured with improved precision and extended to

the journal of chemical physics

Infrared laser absorption spectroscopy of the ν4(σ<i>u</i>) fundamental and associated ν11(π<i>u</i>) hot band of C7: Evidence for alternating rigidity in linear carbon clusters

Infrared laser absorption spectroscopy of the ν4(σu) fundamental and associated ν11(πu) hot band of C7: Evidence for alternating rigidity in linear carbon clusters