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The classical Becker–Doering theory has predicted to within 5% the critical supersaturations required for homogeneous nucleation for more than a dozen molecules. These successes have prompted us to investigate whether the classical theory can predict the experimental results for more extreme cases, i.e., high temperature measurements on large, polar molecules with hydrogen‐bonding functional groups, like l‐menthol. It is therefore the purpose of this paper (1) to report high temperature diffusion cloud chamber measurements on 1‐menthol vapor; (2) to present the thermophysical properties, data or calculated values, required for (a) the experiment, i.e., the mass and heat flux equations, (b) the theory, and (c) the film correction; and (3) to compare the predictions of the Becker–Doering theory with the experimental results. Critical supersaturations, measured over the temperature range 41–100 °C, are about 7% higher than those predicted by the theory. Applying a film correction to the raw data brings the e...

Estimation of thermophysical properties of a large polar molecule and application to homogeneous nucleation of l-menthol