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We report an easy-to-implement method that allows the direct generation ofwater-in-water (w/w) single emulsions. The method relies on direct perturbationof the pressure that drives the flow of the dispersed phase of the emulsions.The resultant inner jet is induced to break up into droplets due to the growthof the perturbation through Rayleigh-Plateau instability [L. Rayleigh, Proc. R.Soc. London 29, 71-97 (1879)]; this leads to the formation of monodispersedroplets. By implementing this method on a modified microfluidic device, wedirectly generate water-in-water-in-water (w/w/w) double emulsions with goodcontrol over the size and the number of encapsulated droplets. Our approachsuggests a new route to apply droplet-based microfluidics to completelywater-based systems.

Forced generation of simple and double emulsions in all-aqueous system