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Water is often viewed as a collection of monomers interactingelectrostatically with each other. We compare the water proton momentumdistributions from recent neutron scattering data with those calculated fromtwo electronic structure based models. We find that below 500 K theelectrostatic models are not able to even qualitatively account for the sizablevibrational zero-point contribution to the enthalpy of vaporization. Thisdiscrepancy is evidence that the change in the proton well upon solvationcannot be entirely explained by electrostatic effects alone.

The proton momentum distribution in strongly H-bonded phases of water; a critical test of electrostatic models