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Colossal magnetoresistance (CMR) and electroresistance (CER) induced by theelectric field in spinel multiferroic CdCr2S4 are reported. It is found that ametal-insulator transition (MIT) in CdCr2S4 is triggered by the electricalfield. In magnetic fields, the resistivity of CdCr2S4 responds similarly tothat of CMR manganites. Combing previous reports, these findings make CdCr2S4the unique compound to possess all four properties of the colossalmagnetocapacitive (CMC), colossal electrocapacitive (CEC), CER, and CMR. Thepresent results open a new venue for searching new materials to show CMR bytuning electric and magnetic fields.

Colossal Electroresistance and Colossal Magnetoresistance in Spinel Multiferroic CdCr2S4