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In the quest for novel magnetoelectric materials, we have grown, stabilizedand explored the properties of La3BAlMnO9 (B = Co or Mn) thin films. In thispaper, we report the influence of the growth parameters that promote B/Al/Mnordering in the pseudo-cubic unit cell and their likely influence on themagnetic and multiferroic properties. The temperature dependence of themagnetization shows that La3CoAlMnO9 is ferromagnetic up to 190 K whileLa3NiAlMnO9 shows a TC of 130 K. The behavior of these films are compared andcontrasted with related La2BMnO6 double perovskites. It is observed that theinsertion of AlO6 octahedra between CoO6 and MnO6 suppresses significantly thestrength of the superexchange interaction, spin-phonon and spin-polar coupling.

Phase formation, phonon behavior, and magnetic properties of novel ferromagnetic La3BAlMnO9 (B = Co or Ni) triple perovskites