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A heterostructure comprised of a 2.7 nm (7 unit-cell) thick layer of themetallic ferromagnet La(2/3)Ca(1/3)MnO(3) and two 50 nm thick layers of thehigh-temperature superconductor YBa(2)Cu(3)O(7) epitaxially grown on (100)SrTiO3 by pulsed-laser deposition was characterized by magnetizationmeasurements and spherical-aberration-corrected high-resolution transmissionelectron microscopy (HRTEM). The saturation magnetization is about half of thatin bulk La(2/3)Ca(1/3)MnO(3). A massive reduction of the magnetizationpreviously inferred from sputter-deposited La(2/3)Ca(1/3)MnO(3)-YBa(2)Cu(3)O(7)heterostructures can be ruled out. HRTEM image analysis, combined with imagesimulation and a focus series reconstruction, revealed atomically sharpepitaxial structures with stacking sequences -(La,Ca)O-CuO2- and -BaO-MnO- atthe top and bottom interface.

Magnetic properties and atomic structure of La(2/3)Ca(1/3)MnO(3)-YBa(2)Cu(3)O(7) heterointerfaces