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Charge ordering, dielectric permittivity and local structure ofLa5/3Sr1/3NiO4 system have been explored X-ray charge scattering, complexdielectric impedance spectroscopy, and extended X-ray absorption fine structure(EXAFS) measurements, made on the same single crystal sample. The localstructure measured by the temperature dependent polarized Ni K-edge EXAFS showssignificant distortions in the NiO2 planes. These local distortions could bereasonable cause of high dielectric permittivity of the title system (e=100 at5K) with the charge ordering in this system being a ferroelectric-like secondorder transition.

Charge order, dielectric response and local structure of La5/3Sr1/3NiO4 system