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Ferromagnetic La3NiAlMnO9 (LNAMO) and La3CoAlMnO9 (LCAMO) triple-perovskitethin films are stabilized in the 750-860 oC temperature range in 100 to 900mTorr O2 pressure range using pulsed-laser deposition. The LCAMO and LNAMOfilms exhibit ferromagnetism up to 190 K and 130 K respectively. Thestructural, optical and magnetic properties of these films demonstrate that theB-site 3d-cations, Al, Mn and Co or Ni ions, are structurally short-rangeordered. The strong spin-lattice-polarization coupling in LCAMO is evidenced bythe temperature dependence of the dielectric constant and the softening of thephonon frequencies starting in the vicinity of theferromagnetic-to-paramagnetic phase transition mimicking the behaviours ofLa2CoMnO6 double perovskite.

Stabilization and functional properties of La3NiAlMnO9 and La3CoAlMnO9 magnetoelectric triple perovskites