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Sum frequency generation vibrational spectra of the water molecules at theNaF and KF aqueous solution surfaces showed significantly different spectralfeatures and different concentration dependence. This result is the firstdirect observation of the cation effects of the simple alkali cations, whichhave been believed to be depleted from the aqueous surface, on the hydrogenbonding structure of the water molecules at the electrolyte solution surfaces.These observations may provide important clue to understand the fundamentalphenomenon of ions at the air/water interface.

Spectroscopic Evidence for the Specific Na+ and K+ Interactions with the Hydrogen-bonded Water Molecules at the Electrolyte Aqueous Solution Surfaces