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The surface stabilized MnO(100)-like monolayer, characterised by a regularc(4x2) distribution of Mn vacancies, is studied by hybrid functionals anddiscussed in the light of available scanning tunneling microscopy andhigh-resolution electron energy loss spectroscopy data. We show that the use ofhybrid functionals is crucial to account for the intermingled nature ofmagnetic ineractions, electron localization, structural distortions and surfacephonons. The proposed Pd(100) supported Mn3O4 structure is excellentlycompatible with the experiments previously reported in literature.

Interplay between magnetic, electronic and vibrational effects in monolayer Mn_3O_4 grown on Pd(100)