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We employ the velocity map imaging technique to measure kinetic energy andangular distributions of state selected CH3 (v2=0,1,2,3) and Br (2P3/2,2P1/2)photofragments produced by methyl bromide photolysis at 215.9 nm. These resultsshow unambiguously that the Br and Br* forming channels result in differentvibrational excitation of the umbrella mode of the methyl fragment. Low energystructured features appear on the images which arise from CH3Br+photodissociation near 330 nm. The excess energy of the probe laser photon ischanneled into CH3+ vibrational excitation, most probably in the nu_4degenerate bend

UV photodissociation of methyl bromide and methyl bromide cation studied by velocity map imaging