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We report on the first observation of the photofragmentation dynamics ofSF$_2^+$. With the aid of state-of-the-art ab initio calculations on thelow-lying excited cationic states of SF$_2^+$ performed by Lee et al. [J. Chem.Phys. 125, 104304 (2006)], a predissociation channel of SF$_2^+$ is evidencedby means of resonance-enhanced multilphoton ionization spectroscopy. This workrepresents a second experimental investigation on the low-lying excitedcationic states of SF$_2^+$. [The first one is the He I photoelectron spectrumof SF$_2^+$ reported by de Leeuw et al. three decades ago, see Chem. Phys. 34,287 (1978).]

On the photofragmentation of SF$_2^+$: Experimental evidence for a predissociation channel