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While Pb(Zn1∕3Nb2∕3)O3–PbTiO3 (PZN-PT) single crystals have shown superior ferroelectric properties, less scientific and technical interests have been placed on PZN-PT polycrystalline ceramics due to their poor thermodynamic stability and the difficult processing conditions. Here, we stabilized the PZN-PT based ceramics by adding alkali niobates such as NaNbO3 (NN) and KNbO3 (KN) and investigated their structure and dielectric properties. Two stabilization mechanisms are suggested in alkali niobate added PZN-PT ceramics, increased tolerance factor and enhanced electronegativity difference. KN stabilized the perovskite structure of PZN-PT based ceramics more effectively than NN. Both PZN-PT-KN and PZN-PT-NN ceramics showed the typical behavior of relaxor ferroelectrics. The temperature of maximum dielectric constant of PZN-PT-NN was slightly higher than that of the PZN-PT-KN, which was explained by the difference in ionic size and B-site ordering.

The effect of alkali niobate addition on the phase stability and dielectric properties of Pb(Zn1∕3Nb2∕3)O3 based ceramic