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The partial photoionization cross sections and asymmetry parameters of S atoms have beenmeasured using constant-ionic-state CIS spectroscopy in the photon energy range 10.0–30.0 eV.The ionizations investigated in these CIS experiments are the 3p−1 ionizations S+4S←S3P,S+2D←S3P, and S+2P←S3P. For the first time Rydberg series which converge to the fourthionization limit have been observed and assignments of these series have been proposed. Thesecorrespond to excitations to Rydberg states that are parts of series which converge to the fourthionization limit, S+4P←S3P 3s−1, and autoionize to the lower S+4S, S+2D, or S+2P states.For each series observed in the CIS spectra photoelectron angular distribution studies, combinedwith other evidence, has allowed the angular momentum character of the free electron onautoionization to be determined

the journal of chemical physics

Measurement of the partial photoionization cross sections and asymmetry parameters of S atoms in the photon energy range 10.0–30.0eV using constant-ionic-state spectroscopy