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Epitaxial thin films of Bi2NiMnO6 were synthesized on SrTiO3 substrates by pulsed laser deposition. The resulting film had the rock-salt-type arrangement of Ni2+ and Mn4+ ions in a double-perovskite unit cell. The films clearly showed multiferroic properties, both ferromagnetic behavior with a Curie temperature of about 100K and ferroelectric behavior with a saturated polarization of about 5μC∕cm2.

Multiferroic thin film of Bi2NiMnO6 with ordered double-perovskite structure