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The radio‐frequency and microwave spectra of 6Li127I have been observed by the molecular‐beam electric‐resonance method of molecular spectroscopy. Spectra of 6Li127I in the first two vibrational states were obtained. From the J=1 radio frequency, Stark spectra values were obtained for the electric dipole moment μ, the iodine nuclear quadrupole interaction eqQI, and the iodine spin‐rotation constant cI. The values of these constants are v=0v=1μ (debye)7.4285±0.0017.5120±0.001eqQI (Mc/sec)−198.780 ±0.005−207.453 ±0.010cI (kc/sec)7.7  ±0.47.8  ±0.6.The observation of J=1→J=0 microwave transitions yielded the following rotational constants: B0=15 304.895±0.005 Mc/sec,B1=15 153.316±0.009 Mc/sec.

Radio-Frequency and Microwave Spectra of 6Li127I by the Molecular-Beam Electric-Resonance Method