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An analysis of the spin‐Hamiltonian parameters of dipositive Es (Es III) in cubic sites in CaF2 has shown that for this ion, the ratio of crystalline field parameters − B6 / B4 < 0.21; the orbital reduction factor (1 − k) = 0.033 ± 0.005; and the value of the nuclear moment of 253Es is μN = (+)3.62 ± 0.5 nm, where the sign is obtained from the consideration of nuclear systematics.

Analysis of the Electron Paramagnetic Resonance Spectrum of Divalent Es in CaF2