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The g values of the ground Γ7 state of Pu3+ in cubic symmetry sites in CaF2, SrF2, and BaF2 are 1.297 ± 0.001, 1.250 ± 0.002, and 1.187 ± 0 004, respectively, as measured at T = 1.2°K by EPR techniques. By fitting the g values, estimates of the crystalline‐field parameters are derived. It is shown that crystalline‐field effects for Pu3+ in the alkaline‐earth fluorides are the same order of magnitude as in the lanthanide series.

Electron Paramagnetic Resonance of Pu3+ in Cubic Symmetry Sites in CaF2, SrF2, and BaF2