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A reduced-dimensionality quantum model is proposed to simulate the vibrational predissociation of BC-Rg2 vdW complexes. The model is applied to simulate the predissociation dynamics of Cl2-Ne2. The results are compared to available experimental data and to previous calculations using a reduced-dimensionality quantum model and a full-dimensional quantum-classical approach.© 2001 American Institute of PhysicsThis work was supported by D.G.I.C.Y.T., Spain, Grant No. PB95-0071. One of the authors ~M.C.! acknowledges nancial support for a stay of six months in Madrid to the European network Training and Mobility of Researchers ~TMR!, Grant No. HPRN-CT-1999-00005.Peer Reviewe

the journal of chemical physics

A reduced-dimensionality quantum model which incorporates the full-dimensional energy of the system: Application to the vibrational predissociation of Cl2–Ne2