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Quaternary sediments and soils at the Forsmark site (Sweden) would constitute the last barrier for radionuclide migration interposed between a deep repository of high level nuclear wastes (HLNW) and surface ecological systems. The retention capacity of these sediments is evaluated by means of reactive transport simulations. Two different scenarios have been modelled: (1) Inflow of deep fluids carrying radionuclides into shallow aquifers hosted in the carbonate glacial till, and (2) Inflow of deep fluids carrying radionuclides into organic matter-bearing clays. The model results predict that caesium is very efficiently retained in both scenarios for periods longer than 3000 years due to the strong affinity of this ion with the frayed edge sites of the illite layers. Strontium is also retained via cation exchange in illite and, in a lesser extent, via co-precipitation in calcite. The retention efficiency for strontium, however, quickly decreases to 0 after 1000 years. Uranium is retained in both scenarios with retention efficiencies higher than 40% at long term (>3000 years) due to precipitation of amorphous uraninite and adsorption on Fe(III) oxyhydroxides. Radium is only retained in the till aquifer since co-precipitation with barium sulphate does not occur in the clay porewater.

Modelling the radionuclide transfer from bedrock to surface systems at Forsmark site (Sweden)